I love this scene, where Walt finally has had too much of Skyler and her emasculating bullshit, and her constant underestimating of him. It's also great, for displaying Walt's self destructive pride and his grandiose self image. It really captures their relationship up to that point.
(Episode 4.6, don't watch if you're not there yet)
http://www.youtube.com/watch?v=wMEq1mGpP5A



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